Sky Sports cameras captured Klopp reacting to Spurs’ quick fire double – and Reds fans weren’t impressed as Liverpool slipped two behind in just 12 minutes.
Harry Kane had given the home side the lead in just four minutes before he turned provider and set up his South Korean teammate.
Dejan Lovren, a man who has come under fire for his poor defences performances of late, was at fault for the goal again.
The centre-back had attempted to head away a Hugo Lloris clearance but missed the ball and allowed Kane to get in behind him.
Kane found his teammate in the box, picking him out with a fine cross, and he easily beat Simon Mignolet from close such a range.
It seems the German was merely smirking in disbelief at what he had just witnessed, but that got on the wrong side of few Reds fans who took to social media to express their disgust.